FY 2007 LDRD Director's R&D Progress SummaryProposal Title: Developing a Science Base for Fuel Reprocessing Separations in the Global Nuclear Energy Program

de Almeida, Valmor F ; Tsouris, Costas ; Birdwell Jr, Joseph F ; D' ; Azevedo, Ed F ; Jubin, Robert Thomas ; DePaoli, David W ; Moyer, Bruce A

Oak Ridge National Laboratory

关键词: Reprocessing;    Fluid Flow;    Kinetics;    Mathematical Models;    Nuclear Energy;   

DOI  :  10.2172/1001706
RP-ID  :  ORNL/TM-2007/114
RP-ID  :  DE-AC05-00OR22725
RP-ID  :  1001706

美国|英语

来源: UNT Digital Library

【 摘 要 】

This work is aimed at developing an experimentally validated computational capability for understanding the complex processes governing the performance of solvent extraction devices used for separations in nuclear fuel reprocessing. These applications pose a grand challenge due to the combination of complicating factors in a three-dimensional, turbulent, reactive, multicomponent, multiphase/interface fluid flow system. The currently limited process simulation and scale-up capabilities provides uncertainty in the ability to select and design the separations technology for the demonstration plan of the Global Nuclear Energy Partnership (GNEP) program. We anticipate the development of science-based models for technology development and design. This project will position ORNL to address the emerging opportunity by creating an expandable process model validated experimentally. This project has three major thrusts, namely, a prototype experimental station, a continuum modeling and simulation effort, and molecular modeling and kinetics support. Excellent progress has been made in corresponding activities in this first year in: (1) defining, assembling, and operating a relevant prototype system for model validation; (2) establishing a mathematical model for fluid flow and transport; (3) deploying sub-scale molecular modeling.