Spin-gap evolution upon Ca doping in the spin-ladder series Sr14-xCaxCu24O41 studied by inelastic neutron scattering

Article

关键词: SUPERCONDUCTIVITY;    SR14CU24O41;    PRESSURE;    DYNAMICS;   

DOI  :  10.1103/PhysRevB.88.014504

来源: SCIE

【 摘 要 】

The spin-gap evolution upon Ca doping in Sr14-xCaxCu24O41 was systematically investigated using inelastic neutron scattering. We discover that the singlet-triplet spin-gap excitation survives in this series with x up to 13, indicating the singlet dimer ground state in these compounds. This observation corrects the previous speculation that the spin gap collapses at x similar to 13 by the NMR technique. The strong intensity modulation along Q(H) in x = 0 gradually evolves into a Q-independent feature in x > 11. This could be attributed to the localized Cu moment magnetism developing into an itinerant magnetism with increasing x. It is a surprise that the spin gap persists in the normal state of this spin-ladder system with metallic behavior, which evidences the possibility of magnetically mediated carrier pairing mechanism in a two-leg spin-ladder lattice.

【 授权许可】

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