科技报告详细信息
Tritium Movement and Accumulation in the NGNP System Interface and Hydrogen Plant
Ohashi, Hirofumi ; Sherman, Steven R.
Idaho National Laboratory
关键词: Water Hydrogen;    Heat Transfer;    Electrolysis;    Isotopic Exchange;    Tritium;   
DOI  :  10.2172/919556
RP-ID  :  INL/EXT-07-12746
RP-ID  :  DE-AC07-99ID-13727
RP-ID  :  919556
美国|英语
来源: UNT Digital Library
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【 摘 要 】

Tritium movement and accumulation in a Next Generation Nuclear Plant with a hydrogen plant using a high temperature electrolysis process and a thermochemical water splitting sulfur iodine process are estimated by the numerical code THYTAN as a function of design, operational, and material parameters. Estimated tritium concentrations in the hydrogen product and in process chemicals in the hydrogen plant of the Next Generation Nuclear Plant using the high temperature electrolysis process are slightly higher than the drinking water limit defined by the U.S. Environmental Protection Agency and the limit in the effluent at the boundary of an unrestricted area of a nuclear plant as defined by the U.S. Nuclear Regulatory Commission. However, these concentrations can be reduced to within the limits through use of some designs and modified operations. Tritium concentrations in the Next Generation Nuclear Plant using the Sulfur-Iodine Process are significantly higher as calculated and are affected by parameters with large uncertainties (i.e., tritium permeability of the process heat exchanger, the hydrogen concentration in the heat transfer and process fluids, the equilibrium constant of the isotope exchange reaction between HT and H2SO4). These parameters, including tritium generation and the release rate in the reactor core, should be more accurately estimated in the near future to improve the calculations for the NGNP using the Sulfur-Iodine Process. Decreasing the tritium permeation through the heat exchanger between the primary and secondary circuits may be an an effective measure for decreasing tritium concentrations in the hydrogen product, the hydrogen plant, and the tertiary coolant.

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