Preparation of Small Well Characterized Plutonium Oxide Reference Materials and Demonstration of the Usefulness of Such Materials for Nondestructive Analysis

Guillen, B.A. ; Hsue, S.T. ; Huang, J.Y ; Hypes, P.A. ; Long, S.M. ; Rudy, C.R. ; Russo, P.A. ; Stewart, J.E. ; Temer, D.J.

Los Alamos National Laboratory

关键词: Calibration;    Calorimetry;    Nondestructive Analysis;    Multiplicity;    Geometry;   

DOI  :  10.2172/807111
RP-ID  :  LA-13991
RP-ID  :  W-7405-ENG-36
RP-ID  :  807111

美国|英语

来源: UNT Digital Library

【 摘 要 】

Calibration of neutron coincidence and multiplicity counters for passive nondestructive analysis (NDA) of plutonium requires knowledge of the detector efficiency parameters. These are most often determined empirically. Bias from multiplication and unknown impurities may be incurred even with small plutonium metal samples. Five sets of small, pure plutonium metal standards prepared with well-known geometry and very low levels of impurities now contribute to determining accurate multiplication corrections. Recent measurements of these metal standards, with small but well-defined multiplication and negligible yield of other than fission neutrons, demonstrate an improved characterization and calibration of neutron coincidence/multiplicity counters. The precise knowledge of the mass and isotopic composition of each standard also contributes significantly to verifying the accuracy of the most precise calorimetry and gamma-ray spectroscopy measurements.