Lithium solid-state batteries: State-of-the-art and challenges for materials, interfaces and processing

JOURNAL OF POWER SOURCES

卷:502

Article

Boaretto, Nicola¹  Garbayo, Inigo¹  Valiyaveettil-SobhanRaj, Sona^1,2  Quintela, Amaia^1,2  Li, Chunmei¹  Casas-Cabanas, Montse^1,3  Aguesse, Frederic¹ 

[1] Basque Res & Technol Alliance BRTA, Ctr Cooperat Res Alternat Energies CIC energiGUNE, Alava Technol Pk,Albert Einstein 48, Vitoria 01510, Spain

[2] Univ Basque Country UPV EHU, Barrio Sarriena S-N, Leioa 48940, Spain

[3] Ikerbasque, Basque Fdn Sci, Maria Diaz de Haro 3, Bilbao 48013, Spain

关键词: Solid state batteries;    Processing technology;    Interfacial challenges;    Solid electrolytes;   

DOI  :  10.1016/j.jpowsour.2021.229919

来源: Elsevier

【 摘 要 】

Lithium solid-state batteries (SSBs) are considered as a promising solution to the safety issues and energy density limitations of state-of-the-art lithium-ion batteries. Recently, the possibility of developing practical SSBs has emerged thanks to striking advances at the level of materials; such as the discovery of new highly-conductive solid-state electrolytes. Consequently, the focus in research has progressively shifted towards the integration of the various components, the battery's functionality at full cell level, and the scalability of the fabrication processes. Considering these points, the development of SSBs still faces formidable challenges. This review covers the recent advances in SSB development, stressing the importance of full cell integration. The most relevant materials and fabrication processes are briefly summarized and their potential applications in SSBs are examined. The main challenges and strategies for full cell integration are then discussed highlighting the most promising materials and the best suited processing techniques. Particular attention is paid on the mutual compatibility of the cell components, the properties of the interfaces within the cell (anode-electrolyte, cathode-electrolyte, intraelectrolyte) and the strategies applied to stabilize and minimize the resistance of these interfaces via compatible processing.

【 授权许可】

Free