Direct observation of double exchange in ferromagnetic La0.7Sr0.3CoO3 by broadband ellipsometry | |
Article | |
关键词: OPTICAL CONDUCTIVITY; ELECTRONIC-STRUCTURE; TRANSITION; TEMPERATURE; MANGANITES; | |
DOI : 10.1103/PhysRevB.97.045137 | |
来源: SCIE |
【 摘 要 】
We present results of our broadband ellipsometry measurements of the optical response of ferromagnetic La0.7Sr0.3CoO3. Our data show that the ferromagnetic transition is accompanied by a transfer of optical spectral weight from an absorption band centered at 1.5 eV to a narrow component of the Drude-like peak. The associated reduction of the intraband kinetic energy is significantly larger than k(B)T(c), confirming that the double exchange plays a major role in the ferromagnetism of doped cobaltites. In conjunction with results of recent theoretical studies, the temperature dependence of the Drude-like peak suggests that the double exchange is mediated by t(2g) orbitals.
【 授权许可】
Free