The Salt Waste Processing Facility and the Actinide Removal Process at the Savannah River Site will remove alpha emitting radioisotopes from High Level Waste to meet regulatory disposal requirements. The removal occurs prior to removal of the radioactive cesium. Both facility designs currently include verification measurement using conventional wet chemistry approaches remote from the operation. Use of an on-line monitor for this purpose offers the opportunity to shorten process cycle time and thereby increase facility throughput.