Novel Composite Hydrogen-Permeable Membranes for Non-Thermal Plasma Reactors for the Decomposition of Hydrogen Sulfide. Quarterly Report April 1-June 30, 2004.
Argyle, M. D. ; Ackerman, J. F. ; Muknahallipatna, S. ; Hamann, J. C. ; Legowski, S.
The goal of this experimental project is to design and fabricate a reactor and membrane test cell to dissociate hydrogen sulfide (H2S) in a non-thermal plasma and recover hydrogen (H2) through a superpermeable multi-layer membrane. Superpermeability of hydrogen atoms (H) has been reported by some researchers using membranes made of Group V transition metals (niobium, tantalum, vanadium, and their alloys), although it has yet to be confirmed in this study. Experiments involving methane conversion reactions were conducted with a preliminary pulsed corona discharge reactor design in order to test and improve the reactor and membrane designs using a non-toxic reactant.