Underwater Analysis of Irradiated Reactor Slugs for CO-60 and Other Radionuclides at the Savannah River Site.

Casella, V. R. ; Salaymeh, S. R. ; Moore, F. S. ; Sigg, R. A. ; Hallford, B. S. ; Osteen, R. S.

Technical Information Center Oak Ridge Tennessee

关键词: Radionuclides;    Irradiation;    Sodium iodides;    Gamma detection;    Plutonium isotopes;   

RP-ID  :  DE2004824526

学科分类：工程和技术（综合）

美国|英语

来源: National Technical Reports Library

【 摘 要 】

Co-60 was produced in the Savannah River Site (SRS) reactors in the 1970s, and the irradiated cobalt reactor slugs were stored in a reactor basin at SRS. Since the activity rates of these slugs were not accurately known, assaying was required. A sodium iodide gamma detector was placed above a specially designed air collimator assembly, so that the slug was eight to nine feet from the detector and was shielded by the basin water. Also, 18 curium sampler slugs, used to produce Cm-244 from Pu-239, were to be disposed of with the cobalt slugs. The curium slugs were also analyzed with a High Purity Germanium (HPGE) detector in an attempt to identify any additional radionuclides produced from the irradiation. Co-60 concentrations were determined for reactor disassembly basin cobalt slugs and the 18 curium sampler slugs. The total Co-60 activity of all of the assayed slugs in this work summed to 31,783 curies on 9/15/03. From the Co-60 concentrations of the curium sampler slugs, the irradiation flux was determined for the known irradiation time. The amounts of Pu-238,-239,-240,-241,-242; Am-241,-243; and Cm-242,-244 produced were then obtained based on the original amount of Pu-239 irradiated.