The Department of Energy (DOE), National Spent Nuclear Fuel Program (NSNFP) has the responsibility to provide the Yucca Mountain Project (YMP) with information on the release of fission products and actinides from DOE spent fuels, which include fast-flux MOX fuel. The nuclide release behavior of two MOX fuel pins, which had high centerline temperatures (210O degrees C) during irradiation and steep temperature gradients across the 3-mm radius of the fuel pin, i.e. from 21OO degrees C to 600 degrees C, are being examined under unsaturated conditions. The high centerline temperature during irradiation resulted in massive grain restructuring with the formation of columnar grains at the center to mid-radius of a pin and equiaxed grains adjacent to the columnar grains.