The Rayleigh scattering signal from femtosecond laser pulses is examined for its utility at making instantaneous density measurements in the NASA Langley 0.3-m Transonic Cryogenic Tunnel. An electron-multiplying CCD camera is used to visualize Rayleigh scattering signal taken concurrently with velocity measurements utilizing the femtosecond laser tagging velocimetry technique (FLEET). The results indicate a strong potential for making instantaneous measurements. Viable single-shot images are obtained over the full operational envelope of the facility, and shot-to-shot variations are found to be on average 6 percent (at 95 percent confidence level) and tend to decrease as the facility density is increased. The Rayleigh scattering signals observed before the optical focus exhibit a characteristically linear dependence on the mass-density of the gas, while signals after the focus exhibit a nonlinear (sublinear) density dependence, indicative of stronger absorption at higher densities. The measured Rayleigh scattering signals compare favorably to theoretical assessments made at the tunnel operating conditions.
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