Activity Estimates of Various Radionuclides in Saltstone Vapor Phase

MILES, DENHAM

Savannah River Site (S.C.)

关键词: Antimony;    36 Materials Science;    Gases;    Tin Isotopes;    Radioisotopes;   

DOI  :  10.2172/838833
RP-ID  :  WSRC-TR-2005-00046
RP-ID  :  AC09-96SR18500
RP-ID  :  838833

美国|英语

来源: UNT Digital Library

【 摘 要 】

Savannah River National Laboratory estimated activities of various radionuclides in vapor phase associated with saltstone. These radionuclides, as well as the estimated activity and concentration of each in the gases phase are listed. Some of the activities are so low they should be considered zero. In particular, activity of the antimony and tin isotopes in the gas phase correspond to less than a molecule of gas per 340 m3 of vapor volume. Equilibrium calculations of the partitioning of each radionuclide between vapor and dissolved phases were done using the Geochemists Workbench (R). The conceptual model used was that 1 curie of each constituent was available to partition between vapor and dissolved phases. The overall assumption is that exposure would come from a single release of the vapor phase from a saltstone vault.