2002 Initial Assessments for B-BX-BY Field Investigation Report (FIR): Numerical Simulations

Freedman, Vicky L. ; Williams, Mark D. ; Cole, C. R. ; White, Mark D. ; Bergeron, Marcel P.

Pacific Northwest National Laboratory (U.S.)

关键词: Technetium 99;    Solutes;    Contaminant Transport;    Waste Management;    Nitrates;   

DOI  :  10.2172/15002644
RP-ID  :  PNNL-13949
RP-ID  :  AC05-76RL01830
RP-ID  :  15002644

美国|英语

来源: UNT Digital Library

【 摘 要 】

IIn support of CH2M HILL Hanford Group, Inc.'s (CHG) preparation of a Field Investigative Report (FIR) for the Hanford Site Single-Shell Tank (SST) Waste Management Area (WMA) B-BX-BY, a set of numerical simulations of flow and solute transport was executed to predict the performance of surface barriers for reducing long-term risks from potential groundwater contamination at the B-BX-BY WMA. This report documents the simulation of 14 cases involving two-dimensional cross sections through the B-BX-BY WMA. Two cross-sections were used for this analysis, one through the BX WMA from tanks BX-108 to BX-102, and another through the trench B-38 for simulating B trench discharges. The simulations were used to investigate the impact of surface barriers, water-line leaks, inventory placement, meteoric recharge and partitioning between the aqueous and sorbed phases. Three transported solutes were considered: uranium-238 (U-238), technetium-99 (Tc-99), and nitrate (NO3). For the BX tank simulations, results showed that simulations investigating water-line leaks demonstrated the highest peak concentrations. Interim barriers had a significant impact on peak concentrations in later times, but not in early times due to a high concentration zone of contaminants near the water table. Overall, simulation results for the BX WMA showed that only a small fraction of the U-238 inventory migrated from the vadose zone in most of the test cases. In general, similar peak WMA concentrations occurred for all of the simulations (<800 pCi/L for Tc-99 and <800 mg/L for NO3), with the exception of the water-line leak cases. In the B trench cases, simulations predicted that the U-238 would not migrate from the vadose zone to the aquifer in the thousand years that were simulated. The simulations also predicted that Tc-99 would appear quickly in the aquifer following the trench discharge in 1954, with peak concentrations occurring around 2020 to 2030.