CHARACTERIZATION OF TANK 5F VERTICAL COOLING COIL LEACHATES FOR SELECT RADIONUCLIDES 2011

Oji, L. ; Diprete, D.

Savannah River Site (S.C.)

关键词: Corrosion;    Leaching;    Americium 241;    Sensitivity;    Leachates;   

DOI  :  10.2172/1025520
RP-ID  :  SRNL-STI-2011-00372
RP-ID  :  DE-AC09-08SR22470
RP-ID  :  1025520

美国|英语

来源: UNT Digital Library

【 摘 要 】

Two twenty-four inch samples of vertical sections of the cooling coils from Tank 5F, taken from Riser 1, were made available to SRNL by SRR for leaching and characterization of the leachates for select radionuclide trapped in the corrosion layer on the exterior of the cooling coils. One piece of cooling coil sample was obtained from a section of a vertical cooling coil located above the 45-inch elevation from the tank floor and the other also from a vertical section of a cooling coil located below the 45-inch elevation from the tank floor of Tank 5F. Analysis results from both cooling coils show that the predominant radionuclides contributing to the activity in both coils are strontium-90 and cesium-137. The activities for strontium-90 and cesium-137 in the Tank 5F vertical cooling coil located above the 45-inch elevation of the tank and designated as sample 5-R1-A45 averaged 1.34E-02 {+-} 1.12E-03 and 7.27E-04 {+-} 4.46E-05 Ci/ft{sup 2}, respectively, while the activities for the vertical cooling coil located below the 45-inch elevation of the tank and designated as sample 5-R1-B45 averaged 8.93E-03 {+-} 8.25E-04 for Sr-90 and 8.10E-04 {+-} 6.36E-05 Ci/ft{sup 2} for Cs-137. Other significant activity contributing radionuclides are americium-241 and europium-154/155. With the exception of the analysis result for Pu-241 in the 5-R1-A45 cooling coils samples, the target detection limits for the other radionuclides were met in both cooling coil samples. The detection limits for Pu-241 analyses result in coil sample 5-R1-A45 were not met consistently because of possible background changes during counting.