Description of Transmutation Library for Fuel Cycle System Analyses

Steven J. Piet ; Samuel E. Bays ; Edward A. Hoffman

关键词: BURNUP;    CONVERSION RATIO;    CROSS SECTIONS;    FAST REACTORS;    FISSION;    FUEL CYCLE;    GLASS;    PROGENY;    TRANSITION ELEMENTS;    TRANSMUTATION;    WASTE FORMS;    WASTES fuel cycle;    reactor physics;    transmutation;   

DOI  :  10.2172/991894
RP-ID  :  INL/EXT-10-19545
PID  :  OSTI ID: 991894
Others  :  TRN: US1007647

学科分类：核能源与工程

美国|英语

来源: SciTech Connect

【 摘 要 】

This report documents the Transmutation Library that is used in Fuel Cycle System Analyses. This version replaces the 2008 version.[Piet2008] The Transmutation Library has the following objectives: ??? Assemble past and future transmutation cases for system analyses. ??? For each case, assemble descriptive information such as where the case was documented, the purpose of the calculation, the codes used, source of feed material, transmutation parameters, and the name of files that contain raw or source data. ??? Group chemical elements so that masses in separation and waste processes as calculated in dynamic simulations or spreadsheets reflect current thinking of those processes. For example, the CsSr waste form option actually includes all Group 1A and 2A elements. ??? Provide mass fractions at input (charge) and output (discharge) for each case. ??? Eliminate the need for either ???fission product other??? or ???actinide other??? while conserving mass. Assessments of waste and separation cannot use ???fission product other??? or ???actinide other??? as their chemical behavior is undefined. ??? Catalog other isotope-specific information in one place, e.g., heat and dose conversion factors for individual isotopes. ??? Describe the correlations for how input and output compositions change as a function of UOX burnup (for LWR UOX fuel) or fast reactor (FR) transuranic (TRU) conversion ratio (CR) for either FR-metal or FR-oxide. This document therefore includes the following sections: ??? Explanation of the data set information, i.e., the data that describes each case. In no case are all of the data presented in the Library included in previous documents. In assembling the Library, we return to raw data files to extract the case and isotopic data, into the specified format. ??? Explanation of which isotopes and elements are tracked. For example, the transition metals are tracked via the following: two Zr isotopes, Zr-other, Tc99, Tc-other, two Mo-Ru-Rh-Pd isotopes, Mo-Ru-Rh-Pd-other, four other specific TM isotopes, and TM-other. Mo-Ru-Rh-Pd are separated because their content constrains the loading of waste in glass, so we have to know the mass of those elements independent of others. ??? Rules for collapsing long lists of isotopes (~1000) to the 81 items in the library. For each tracked isotope, we define which short-lived isotopes??? mass (at t=0) is included with the mass of the tracked isotope at t=0, which short-lived radioactive progeny must be accounted for when the tracked isotope decays, and to which of the other 80 items the mass of the tracked isotope goes when it decays. ??? Explanation of where raw data files can be found on the fuel cycle data portal. ??? Explanation of generic cross section sets ??? Explanation of isotope-specific parameters such as heat and dose conversion factors ??? Explanation of the LWR UOX burnup and FR TRU CR correlations.