High Temperature Fuel Cladding Chemical Interactions Between TRIGA Fuels and 304 Stainless Steel

Perez, Emmanuel¹  Keiser, Jr., Dennis D.¹  Forsmann, Bryan²  Janney, Dawn E.¹  Henley, Jody¹  Woolstenhulme, Eric C.¹ 

[1] Idaho National Lab. (INL), Idaho Falls, ID (United States);Boise State Univ., ID (United States)

关键词: FUEL-CLADDING INTERACTIONS;    STAINLESS STEEL-304;    TRIGA TYPE REACTORS;    TEMPERATURE RANGE 1000-4000 K;    NUCLEAR FUELS;    INCOLOY 800;    CHEMICAL REACTIONS;    UR;   

DOI  :  10.2172/1259949
RP-ID  :  INL/EXT--15-36708
PID  :  OSTI ID: 1259949
Others  :  TRN: US1601536

美国|英语

来源: SciTech Connect

【 摘 要 】

High-temperature fuel-cladding chemical interactions (FCCI) between TRIGA (Training, Research, Isotopes, General Atomics) fuel elements and the 304 stainless steel (304SS) are of interest to develop an understanding of the fuel behavior during transient reactor scenarios. TRIGA fuels are composed of uranium (U) particles dispersed in a zirconium-hydride (Zr-H) matrix. In reactor, the fuel is encased in 304-stainless-steel (304SS) or Incoloy 800 clad tubes. At high temperatures, the fuel can readily interact with the cladding, resulting in FCCI. A number of FCCI can take place in this system. Interactions can be expected between the cladding and the Zr-H matrix, and/or between the cladding and the U-particles. Other interactions may be expected between the Zr-H matrix and the U-particles. Furthermore, the fuel contains erbium-oxide (Er-O) additions. Interactions can also be expected between the Er-O, the cladding, the Zr-H and the U-particles. The overall result is that very complex interactions may take place as a result of fuel and cladding exposures to high temperatures. This report discusses the characterization of the baseline fuel microstructure in the as-received state (prior to exposure to high temperature), characterization of the fuel after annealing at 950C for 24 hours and the results from diffusion couple experiments carries out at 1000C for 5 and 24 hours. Characterization was carried out via scanning electron microscopy (SEM) and transmission electron microscopy (TEM) with sample preparation via focused ion beam in situ-liftout-technique.