Optimization of SHINE Process: Design and Verification of Plant-Scale AG 1 Anion-Exchange Concentration Column and Titania Sorbent Pretreatment

Stepinski, Dominique C.¹  Abdul, Momen¹  Youker, Amanda J.¹  Rotsch, David A.¹  Tkac, Peter¹  Chemerisov, Sergey¹  Vandegrift, George F.¹ 

[1]Argonne National Lab. (ANL), Argonne, IL (United States). Nuclear Engineering Division

关键词: AG1 anion-exchange;    Mo-99;    concentration column;   

DOI  :  10.2172/1314088
RP-ID  :  ANL/NE--16/7
PID  :  OSTI ID: 1314088
Others  :  Other: 129360

美国|英语

来源: SciTech Connect

【 摘 要 】

Argonne National Laboratory has developed a Mo-recovery and -purification system for the SHINE medical technologies process, which uses a uranyl sulfate solution for the accelerator-driven production of Mo-99. The objective of this effort is to reduce the processing time for the acidification of the Mo-99 product prior to loading onto a concentration column and concentration of the Mo-99 product solution. Two methods were investigated: (1) the replacement of the titania concentration column by an anion-exchange column to decrease processing time and increase the radioiodine-decontamination efficiency and (2) pretreatment of the titania sorbent to improve its effectiveness for the Mo-recovery and -concentration columns. Promising results are reported for both methods.