Influence of the accumulation chamber insertion depth to measure surface radon exhalation rates

JOURNAL OF HAZARDOUS MATERIALS

卷:393

Article

Gutierrez-Alvarez, I¹  Guerrero, J. L.¹  Martin, J. E.¹  Adame, J. A.²  Bolivar, J. P.¹ 

[1] Univ Huelva, Res Ctr Nat Resources Hlth & Environm RENSMA, Integrated Sci Dept, Huelva, Spain

[2] Natl Inst Aerosp Technol INTA, Atmospher Res & Instrumentat Branch, Atmospher Sounding Stn El Arenosillo, Mazagon Huelva, Spain

关键词: Radon exhalation;    Accumulation chamber;    Insertion depth;    Phosphogypsum;   

DOI  :  10.1016/j.jhazmat.2020.122344

来源: Elsevier

【 摘 要 】

A common method to measure radon exhalation rates relies on the accumulation chamber technique. Usually, this approach only considers one-dimensional gas transport within the soil that neglects lateral diffusion. However, this lateral transport could reduce the reliability of the method. In this work, several cylindrical-shaped accumulation chambers were built with different heights to test if the insertion depth of the chamber into the soil improves the reliability of the method and, in that case, if it could limit the radon lateral diffusion effects. To check this hypothesis in laboratory, two reference exhalation boxes were manufactured using phosphogypsum from a repository located nearby the city of Huelva, in the southwest of Spain. Laboratory experiments showed that insertion depth had a deep impact in reducing the effective decay constant of the system, extending the interval where the linear fitting can be applied, and consistently obtaining reliable exhalation measurements once a minimum insertion depth is employed. Field experiments carried out in the phosphogypsum repository showed that increasing the insertion depth could reduce the influence of external effects, increasing the repeatability of the method. These experiments provided a method to obtain consistent radon exhalation measurements over the phosphogypsum repository.

【 授权许可】

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