期刊论文详细信息
JOURNAL OF POWER SOURCES 卷:501
The impact of flow field plate misalignment on the gas diffusion layer intrusion and performance of a high-temperature polymer electrolyte fuel cell
Article
Hoppe, Eugen1,2  Janssen, Holger1  Mueller, Martin1  Lehnert, Werner1,2 
[1] Forschungszentrum Julich, IEK 14 Electrochem Proc Engn, Inst Energy & Climate Res, D-52425 Julich, Germany
[2] Rhein Westfal TH Aachen, Modeling Electrochem Proc Engn, D-52062 Aachen, Germany
关键词: Gas diffusion layer;    Membrane electrode assembly;    Misalignment;    Intrusion;    X-ray tomography;    High-temperature polymer electrolyte fuel cell;   
DOI  :  10.1016/j.jpowsour.2021.230036
来源: Elsevier
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【 摘 要 】

Tolerances in the production process of flow field plates for polymer electrolyte fuel cells (PEFCs) and the assembly of single cells and stacks can lead to a misalignment among the flow field plates. Due to clamping and misalignment, shear stresses can be forced on the membrane electrode assembly (MEA). Furthermore, the gas diffusion layer (GDL) intrudes into the channel. In this study, five different degrees of misalignment (0 to 1000 mu m) are applied to a fuel cell model consisting of two flow field plates with five adjacent channels each (1 mm width) and an MEA in between them. For each degree, the MEA is compressed by about 30% and 3D images (tomograms) are recorded using an X-ray computer tomograph (CT). Analyzing the cross-section of the channels, the maximum intrusion depth varies for each channel. Furthermore, the shape of the membrane becomes ever more wavelike, with increasing misalignment and the position of the maximum intrusion depth shifts sideways from the center of the channel. Additionally, high-temperature polymer electrolyte fuel cell (HT-PEFC) single cell experiments are carried out. Two degrees of misalignment are set (normal assembly and 1000 mu m). The performances of both degrees of misalignment are within 5% at a power density of 0.24 W.cm(-2).

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