Redistribution of radionuclides in irradiated AGR-1 UCO TRISO fuel after 1800 °C safety testing

JOURNAL OF NUCLEAR MATERIALS

卷:542

Article

Gerczak, Tyler J.¹  Seibert, Rachel L.^1,2  Hunn, John D.¹  Baldwin, Charles A.¹  Montgomery, Fred C.¹  Morris, Robert N.¹ 

[1] Oak Ridge Natl Lab, Oak Ridge, TN 37830 USA

[2] IIT, Chicago, IL 60616 USA

关键词: TRISO;    AGR;    Post-irradiation examination;    Fission products;    Silicon Carbide;   

DOI  :  10.1016/j.jnucmat.2020.152453

来源: Elsevier

【 摘 要 】

Release of radionuclides from intact tristructural-isotropic (TRISO) coated particle fuel at normal and accident conditions is a primary metric of fuel performance. The distribution of fission products and actinides in the TRISO layers of individual particles provides insight on radionuclide transport and release behavior and was determined using scanning electron microscopy analysis. Particles were isolated from an irradiated fuel compact (AGR-1 Compact 4-4-2) and analyzed as-irradiated or after individual particle safety-testing at 1800 degrees C for 650 h. Particles were selected for comparison based on their remaining Ag-110m fission product inventory. These comparisons corroborated the observation that the Ag-110m inventory is a marker for relative irradiation temperature based on observed radionuclide distribution in the SiC layer. The comparison also indicated that the in-pile behavior influences the fission product and actinide species interactions with the TRISO layers during high temperature exposure after irradiation. The analysis confirms both palladium and uranium diffusion, as well as other species, are active in the UCO TRISO fuel system at 1800 degrees C and that palladium transport is active at lower temperatures relative to uranium. While diffusion across the SiC layer was observed, the intact nature of the SiC layer after the 1800 degrees C, 650-h exposure indicates the SiC layer maintained its functionality as a fission product barrier by mitigating release of radionuclides at beyond accident margin temperatures. (C) 2020 Published by Elsevier B.V.

【 授权许可】

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