In-gas-cell laser ionization studies of plutonium isotopes at IGISOL

NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS

卷:376

Article; Proceedings Paper

Pohjalainen, I.¹  Moore, I. D.¹  Kron, T.²  Raeder, S.^3,4  Sonnenschein, V.⁵  Tomita, H.⁵  Trautmann, N.⁶  Voss, A.¹  Wendt, K.² 

[1] Univ Jyvaskyla, Dept Phys, POB 35 YFL, FI-40014 Jyvaskyla, Finland

[2] Johannes Gutenberg Univ Mainz, Inst Phys, Fritz Strassmann Weg 2, D-55128 Mainz, Germany

[3] Helmholtz Inst Mainz, D-55128 Mainz, Germany

[4] Katholieke Univ Leuven, Inst Kern & Stralingsfys, B-3001 Leuven, Belgium

[5] Nagoya Univ, Chikusa Ku, Furo Cho, Nagoya, Aichi 4648603, Japan

[6] Johannes Gutenberg Univ Mainz, Inst Nucl Chem, Fritz Strassmann Weg 2, D-55128 Mainz, Germany

关键词: Resonance laser ionization;    Gas phase chemistry;    Gas cell;    Plutonium;   

DOI  :  10.1016/j.nimb.2016.02.019

来源: Elsevier

【 摘 要 】

In-gas-cell resonance laser ionization has been performed on long-lived isotopes of Pu at the IGISOL facility, Jyvaskyla. This initiates a new programme of research towards high-resolution optical spectroscopy of heavy actinide elements which can be produced in sufficient quantities at research reactors and transported to facilities elsewhere. In this work a new gas cell has been constructed for fast extraction of laser-ionized elements. Samples of (238-240,242)pu and Pu-244 have been evaporated from Ta filaments, laser ionized, mass separated and delivered to the collinear laser spectroscopy station. Here we report on the performance of the gas cell through studies of the mass spectra obtained in helium and argon, before and after the radiofrequency quadrupole cooler-buncher. This provides valuable insight into the gas phase chemistry exhibited by Pu, which has been additionally supported by measurements of ion time profiles. The resulting monoatomic yields are sufficient for collinear laser spectroscopy. A gamma-ray spectroscopic analysis of the Pu samples shows a good agreement with the assay provided by the Mainz Nuclear Chemistry department. (C) 2016 Elsevier B.V. All rights reserved.

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