Public health impacts of secondary particulate formation from aromatic hydrocarbons in gasoline

Environmental Health

Research

Katherine von Stackelberg¹  Joel A Schwartz¹  Jonathan Buonocore¹  Prakash V Bhave² 

[1] Harvard Center for Risk Analysis, 401 Park Drive, Landmark 404J, 02215, Boston, MA, USA;National Exposure Research Laboratory, Office of Research & Development, U.S. Environmental Protection Agency, 109 T.W. Alexander Dr. Research Triangle Park, 27711, Durham, NC, USA;

关键词: Aromatic hydrocarbons;    Secondary organic aerosol (SOA);    Secondary particulate;    Social cost;    Gasoline;   

DOI  :  10.1186/1476-069X-12-19

 received in 2012-09-05, accepted in 2013-02-13,  发布年份 2013

来源: Springer

【 摘 要 】

BackgroundAromatic hydrocarbons emitted from gasoline-powered vehicles contribute to the formation of secondary organic aerosol (SOA), which increases the atmospheric mass concentration of fine particles (PM2.5). Here we estimate the public health burden associated with exposures to the subset of PM2.5 that originates from vehicle emissions of aromatics under business as usual conditions.MethodsThe PM2.5 contribution from gasoline aromatics is estimated using the Community Multiscale Air Quality (CMAQ) modeling system and the results are compared to ambient measurements from the literature. Marginal PM2.5 annualized concentration changes are used to calculate premature mortalities using concentration-response functions, with a value of mortality reduction approach used to monetize the social cost of mortality impacts. Morbidity impacts are qualitatively discussed.ResultsModeled aromatic SOA concentrations from CMAQ fall short of ambient measurements by approximately a factor of two nationwide, with strong regional differences. After accounting for this model bias, the estimated public health impacts from exposure to PM2.5 originating from aromatic hydrocarbons in gasoline lead to a central estimate of approximately 3800 predicted premature mortalities nationwide, with estimates ranging from 1800 to over 4700 depending on the specific concentration-response function used. These impacts are associated with total social costs of $28.2B, and range from $13.6B to $34.9B in 2006$.ConclusionsThese preliminary quantitative estimates indicate particulates from vehicular emissions of aromatic hydrocarbons demonstrate a nontrivial public health burden. The results provide a baseline from which to evaluate potential public health impacts of changes in gasoline composition.

【 授权许可】

CC BY   
© von Stackelberg et al.; licensee BioMed Central Ltd. 2013