All-coupling polaron optical response: Analytic approaches beyond the adiabatic approximation

Article

关键词: SLOW-ELECTRONS;    ABSORPTION;    CRYSTAL;    TRANSPORT;    MOBILITY;    MOTION;   

DOI  :  10.1103/PhysRevB.94.125206

来源: SCIE

【 摘 要 】

In the present work, the problem of an all-coupling analytic description for the optical conductivity of the Frohlich polaron is treated, with the goal being to bridge the gap in the validity range that exists between two complementary methods: on the one hand, the memory-function formalism and, on the other hand, the strong-coupling expansion based on the Franck-Condon picture for the polaron response. At intermediate coupling, both methods were found to fail as they do not reproduce diagrammatic quantum Monte Carlo results. To resolve this, we modify the memory-function formalism with respect to the Feynman-Hellwarth-Iddings-Platzman approach in order to take into account a nonquadratic interaction in a model system for the polaron. The strong-coupling expansion is extended beyond the adiabatic approximation by including in the treatment nonadiabatic transitions between excited polaron states. The polaron optical conductivity that we obtain at T = 0 by combining the two extended methods agrees well, both qualitatively and quantitatively, with the diagrammatic quantum Monte Carlo results in the whole available range of the electron-phonon coupling strength.

【 授权许可】

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