Nd2Sn2O7: An all-in-all-out pyrochlore magnet with no divergence-free field and anomalously slow paramagnetic spin dynamics

Article

关键词: LOW-TEMPERATURE;    HEISENBERG-FERROMAGNET;    RELAXATION RATE;    GD2SN2O7;    OXIDES;    ANTIFERROMAGNET;    DIFFRACTION;    TRANSITIONS;    FRUSTRATION;    LATTICE;   

DOI  :  10.1103/PhysRevB.92.144423

来源: SCIE

【 摘 要 】

We report measurements performed on a polycrystalline sample of the pyrochlore compound Nd2Sn2O7. It undergoes a second order magnetic phase transition at T-c approximate to 0.91 K to a noncoplanar all-in-all-out magnetic structure of the Nd3+ magnetic moments. The thermal behavior of the low temperature specific heat fingerprints excitations with linear dispersion in a three-dimensional lattice. The temperature independent spin-lattice relaxation rate measured below T-c and the anomalously slow paramagnetic spin dynamics detected up to approximate to 30T(c) are suggested to be due to magnetic short-range correlations in unidimensional spin clusters, i.e., spin loops. The observation of a spontaneous field in muon spin relaxation measurements is associated with the absence of a divergence-free field for the ground state of an all-in-all-out pyrochlore magnet as predicted recently.

【 授权许可】

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