Coexistence of antiferromagnetic ordering and superconductivity in the Ba(Fe0.961Rh0.039)(2)As-2 compound studied by Mossbauer spectroscopy

Article

关键词: HIGH-TEMPERATURE SUPERCONDUCTIVITY;    SPIN-DENSITY-WAVE;    HYPERFINE FIELDS;    IRON;    DISTRIBUTIONS;   

DOI  :  10.1103/PhysRevB.84.024509

来源: SCIE

【 摘 要 】

The results of a Fe-57 Mossbauer spectroscopy study between 2.0 and 294 K of superconducting Ba(Fe0.961Rh0.039)(2)As-2 are reported. The main component of the electric field gradient tensor at 294 K is shown to be positive and its increase with decreasing temperature is well described by a T-3/2 power-law relation. The shape of the Mossbauer spectra below the Neel temperature T-N = 55.5(1) K is shown to result from the presence of doping-induced disorder rather than of incommensurate spin-density-wave order. The measured hyperfine magnetic field reaches its maximum value at the critical temperature T-c = 14 K and then decreases by 4.2% upon further cooling to 2.0 K. This constitutes direct evidence of the coexistence of and competition between superconductivity and magnetic order. The extrapolated value of the Fe magnetic moment at 0 K is determined to be 0.35(1) mu(B). The Debye temperature of Ba(Fe0.961Rh0.039)(2)As-2 is found to be 357(3) K.

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