Resonating valence-bond state in an orbitally degenerate quantum magnet with dynamical Jahn-Teller effect

Article

关键词: TRIANGULAR LATTICE;    SPIN;    HONEYCOMB;    LINIO2;    LIQUID;    ORDER;   

DOI  :  10.1103/PhysRevB.91.045117

来源: SCIE

【 摘 要 】

Short-range resonating valence-bond states in an orbitally degenerate magnet on a honeycomb lattice are studied. A quantum-dimer model is derived from the Hamiltonian which represents the superexchange interaction and the dynamical Jahn-Teller (JT) effect. We introduce two local units termed spin-orbital singlet dimer, where two spins in a nearest-neighbor bond form a singlet state associated with an orbital polarization along the bond, and local JT singlet, where an orbital polarization is quenched due to the dynamical JT effect. A derived quantum-dimer model consists of the hopping of the spin-orbital singlet dimers and the JT singlets, and the chemical potential of the JT singlets. We analyze the model by the mean-field approximation, and find that a characteristic phase, termed JT liquid phase, where both the spin-orbital singlet dimers and the JT singlets move quantum mechanically, is realized. Possible scenarios for the recently observed non-magnetic-ordered state in Ba3CuSb2O9 are discussed.

【 授权许可】

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