Bulk superconductivity at 84 K in the strongly overdoped regime of cuprates

Article

关键词: ELECTRONIC SPECIFIC-HEAT;    CRITICAL-TEMPERATURE;    SUPERFLUID DENSITY;    COPPER OXIDES;    YBA2CU3O7-DELTA;    DEPENDENCE;    OXYGEN;    MO;    TC;   

DOI  :  10.1103/PhysRevB.94.180509

来源: SCIE

【 摘 要 】

By means of magnetization, specific heat, and muon-spin relaxation measurements, we investigate newly synthesized high-pressure oxidized Cu0.75Mo0.25Sr2YCu2O7.54, in which overdoping is achieved up to p similar to 0.46 hole/Cu, well beyond the T-c-p superconducting dome of cuprates, where Fermi-liquid behavior is expected. Surprisingly, we find bulk superconductivity with T-c = 84 K and superfluid density similar to those of optimally doped YBa2Cu3O7-delta. On the other hand, specific heat data display a large electronic contribution at low temperature, comparable to that of nonsuperconducting overdoped La2-x SrxCuO4. These results point at an unusual high-T-c phase with a large fraction of unpaired holes. Further experiments may assess the Fermi-liquid properties of the present phase, which would put into question the paradigm that the high T-c of cuprates originates from a non-Fermi-liquid ground state.

【 授权许可】

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