Phonon-induced long-lasting nonequilibrium in the electron system of a laser-excited solid

Article

关键词: ULTRASHORT LASER;    DYNAMICS;    METALS;    THERMALIZATION;    FEMTOSECOND;    ABLATION;    EXCITATION;    MECHANISMS;    SURFACE;    COPPER;   

DOI  :  10.1103/PhysRevB.99.174314

来源: SCIE

【 摘 要 】

Electron-electron thermalization and electron-phonon relaxation processes in laser-excited solids are often assumed to occur on different timescales. This is true for the majority of the conduction band electrons in a metal. However, electron-phonon interactions can influence the thermalization process of the excited electrons. We study the interplay of the underlying scattering mechanisms for the case of a noble metal with help of a set of complete Boltzmann collision integrals. We trace the transient electron distribution in copper and its deviations from a Fermi-Dirac distribution due to the excitation with an ultrashort laser pulse. We investigate the different stages of electronic nonequilibrium after an excitation with an ultrashort laser pulse of 800 nm wavelength and 10 fs pulse duration. Our calculations show a strong nonequilibrium during and directly after the end of the laser pulse. Subsequently, we find a fast thermalization of most electrons. Surprisingly, we observe a long-lasting nonequilibrium, which can be attributed to the electron-phonon scattering. This nonequilibrium establishes at energies around peaks in the density of states of the electrons and persists on the timescale of electron-phonon energy relaxation. It influences in turn the electron phonon coupling strength.

【 授权许可】

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