Magnetic properties and magnetic structure of the frustrated quasi-one-dimensional antiferromagnet SrCuTe2O6

Article

关键词: QUANTUM SPIN LIQUID;    STATE;    EXCITATIONS;    MONOPOLES;    ANYONS;    CHAINS;   

DOI  :  10.1103/PhysRevB.102.134407

来源: SCIE

【 摘 要 】

Magnetization measurements on single-crystal cubic SrCuTe2O6 with an applied magnetic field along three inequivalent high symmetry directions [100], [110], and [111] reveal weak magnetic anisotropy. The fits of the magnetic susceptibility to the result from a quantum Monte Carlo simulation on the Heisenberg spin-chain model, where the chain is formed via the dominant third-nearest-neighbor exchange interaction J(3), yield the intrachain interaction (J(3)/k(B)) between 50.12(7) K for the applied field along [110] and 52.5(2) K along [100] with about the same g factor of 2.2. Single-crystal neutron diffraction unveils the transition to the magnetic ordered state as evidenced by the onset of the magnetic Bragg intensity at T-N1 = 5.25(9) K with no anomaly of the second transition at T-N2 reported previously. Based on irreducible representation theory and magnetic space group analysis of powder and single-crystal neutron diffraction data, the magnetic structure in the Shubnikov space group P4(1)32, where the Cu2+ S = 1/2 spins antiferromagnetically align in the direction perpendicular to the spin chain, is proposed. The measured ordered moment of 0.52(6) mu(B), which represents 48% reduction from the expected value of 1 mu(B), suggests the remaining influence of frustration resulting from the J(1) and J(2) bonds.

【 授权许可】

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