Spaser quenching by off-resonant plasmon modes

Article

关键词: SINGLE-MOLECULE FLUORESCENCE;    METAL-ENHANCED FLUORESCENCE;    GOLD NANOPARTICLES;    QUANTUM DOTS;    TOY MODEL;    EMISSION;    FLUOROPHORES;    DEPENDENCE;    GRAPHENE;    LASERS;   

DOI  :  10.1103/PhysRevB.96.075423

来源: SCIE

【 摘 要 】

We study the effect of off-resonant plasmon modes on spaser threshold in nanoparticle-based spasers. We develop an analytical semiclassical model and derive spaser threshold condition accounting for gain coupling to higher-order plasmons. We show that such a coupling originates from inhomogeneity of gain distribution near the metal surface and leads to an upward shift of spaser frequency and population inversion threshold. This effect is similar, albeit significantly weaker, to quenching of plasmon-enhanced fluorescence near metal nanostructures due to excitation of off-resonant modes with wide spectral band. We also show that spaser quenching is suppressed for high gain concentrations and establish a simple criterion for quenching onset, which we support by numerical calculations for spherical geometry.

【 授权许可】

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