Recent Progress of Metal Organic Frameworks-Based Electrocatalysts for Hydrogen Evolution, Oxygen Evolution, and Oxygen Reduction Reaction

Energy & Environmental Materials

article

Yaling Jia¹  Ziqian Xue²  Yinle Li¹  Guangqin Li¹ 

[1] MOE Laboratory of Bioinorganic and Synthetic Chemistry, Lehn Institute of Functional Materials, School of Chemistry, Sun Yat-Sen University;Institute for Integrated Cell-Material Sciences ,(iCeMS), Kyoto University

关键词: electrocatalysts;    hydrogen evolution;    metal organic frameworks;    oxygen evolution;    oxygen reduction reaction;   

DOI  :  10.1002/eem2.12290

来源: Wiley

【 摘 要 】

Exploring efficient and cost-saving electrocatalysts is essential to the renewable energy storage and utilization, which is still in its embryonic period. MOFs have drawn tremendous attention due to their adjustability, abundant active sites, and plentiful pores. Notably, satisfactory electrocatalytic performance has been achieved by MOFs-based electrocatalysts comparable to traditional electrocatalysts. State-of-the-art works about the MOFs-based electrocatalysts for hydrogen evolution reaction (HER), oxygen evolution reaction (OER), and ORR were summarized in this review. This review comprises a series of modifying strategies of MOFs and their derivatives, from aspects of structure, composition, and morphology. Furthermore, the active sites and functional mechanisms’ recognition are involved in this review expecting to provide reference for rationally designing efficient electrocatalysts. At last, the current status, challenges, and perspectives of MOFs-based electrocatalysts are also discussed.

【 授权许可】

Unknown