Refining the contribution of riverine particulate release to the global marine Nd budget

Progress in Earth and Planetary Science

Hong Che¹  Jing Zhang¹  Qian Liu¹  Huijun He¹  Zhi-Qi Zhao² 

[1] Frontiers Science Center for Deep Ocean Multispheres and Earth System, and Key Laboratory of Marine Chemistry Theory and Technology, Ministry of Education, Ocean University of China;School of Earth Science and Resources, Chang’an University;

关键词: Particulate release;    Nd budget;    Rare earth elements;    Changjiang estuary;   

DOI  :  10.1186/s40645-022-00479-2

来源: DOAJ

【 摘 要 】

Abstract The release of neodymium (Nd) from particles along continental margins may contribute to losses in the global of Nd budget. The Changjiang River, which carries a heavy load of total suspended matter, empties into the East China Sea, and a strong particulate–seawater interaction process occurs along the salinity gradient. In the low-salinity region (S < 2.0), strong removal of dissolved rare earth elements (dREEs) occurs, but the Nd isotope values are uniform. At mid- and high-salinity (S = 2.0–28.0 and S > 28.0) areas, the dREE concentrations increase slightly. An Nd isotope mass balance indicates that the release of particulate matter is a source of dREEs in the Changjiang estuary. The release rate of particulate Nd (NdSPM) to the dissolved Nd pool in Changjiang estuary is higher than other estuaries, such as Amazon estuary. Composite all river data available from the previous studies indicate that 5800–9200 Mg per year of Nd is released to global marine waters from riverine particles. This estimated quantity is on the same order of magnitude as the calculated global Nd release flux based on the case study in the Amazon estuary. Our study indicates that to better constrain the global Nd budget, it is required to consider the release rate of NdSPM in different rivers due to the significant difference among various rivers, but with very limited available data as of now.

【 授权许可】

Unknown