Intercomparison of arctic XH 2 O observations from three ground-based Fourier transform infrared networks and application for satellite validation

Atmospheric Measurement Techniques Discussions

article

Tu, Qiansi¹  Khosrawi, Farahnaz¹  Sommer, Michael²  Borsdorff, Tobias³  Raffalski, Uwe⁴  Hase, Frank¹  Blumenstock, Thomas¹  Schneider, Matthias¹  Schneider, Andreas³  Kivi, Rigel⁵  Heikkinen, Pauli⁵  Ertl, Benjamin¹  Diekmann, Christopher¹ 

[1] Karlsruhe Institute of Technology (KIT), Institute of Meteorology and Climate Research – Atmospheric Trace Gases and Remote Sensing (IMK-ASF);GRUAN Lead Centre;SRON Netherlands Institute for Space Research;Swedish Institute of Space Physics;Finnish Meteorological Institute;Karlsruhe Institute of Technology, Steinbuch Centre for Computing (SCC)

DOI  :  10.5194/amt-14-1993-2021

学科分类：大气科学

来源: Copernicus Publications

【 摘 要 】

In this paper, we compare column-averaged dry-air mole fractions of water vapor ( XH 2 O ) retrievals from the COllaborative Carbon Column Observing Network (COCCON) with retrievals from two co-located high-resolution Fourier transform infrared (FTIR) spectrometers as references at two boreal sites, Kiruna, Sweden, and Sodankylä, Finland, from 6 March 2017 to 20 September 2019. In the framework of the Network for the Detection of Atmospheric Composition Change (NDACC), an FTIR spectrometer is operated at Kiruna. The H 2 O product derived from these observations has been generated with the MUlti-platform remote Sensing of Isotopologues for investigating the Cycle of Atmospheric water (MUSICA) processor. In Sodankylä, a Total Carbon Column Observing Network (TCCON) spectrometer is operated, and the official XH 2 O data as provided by TCCON are used for this study. The datasets are in good overall agreement, with COCCON data showing a wet bias of ( 49.20±58.61 ) ppm (( 3.33±3.37 ) %, R 2 =0.9992 ) compared with MUSICA NDACC and ( 56.32±45.63 ) ppm (( 3.44±1.77 ) %, R 2 =0.9997 ) compared with TCCON. Furthermore, the a priori H 2 O volume mixing ratio (VMR) profiles (MAP) used as a priori information in the TCCON retrievals (also adopted for COCCON retrievals) are evaluated with respect to radiosonde (Vaisala RS41) profiles at Sodankylä. The MAP and radiosonde profiles show similar shapes and a good linear correlation of integrated XH 2 O , indicating that MAP is a reasonable approximation of the true atmospheric state and an appropriate choice for the scaling retrieval methods as applied by COCCON and TCCON. COCCON shows a reduced dry bias ( −14.96  %) in comparison with TCCON ( −19.08  %) with respect to radiosonde XH 2 O . Finally, we investigate the quality of satellite data at high latitudes. For this purpose, the COCCON XH 2 O is compared with retrievals from the Infrared Atmospheric Sounding Interferometer (IASI) generated with the MUSICA processor (MUSICA IASI) and with retrievals from the TROPOspheric Monitoring Instrument (TROPOMI). Both paired datasets generally show good agreement and similar correlations at the two sites. COCCON measures 4.64 % less XH 2 O at Kiruna and 3.36 % less at Sodankylä with respect to MUSICA IASI, whereas COCCON measures 9.71 % more XH 2 O at Kiruna and 7.75 % more at Sodankylä compared with TROPOMI. Our study supports the assumption that COCCON also delivers a well-characterized XH 2 O data product. This emphasizes that this approach might complement the TCCON network with respect to satellite validation efforts. This is the first published study where COCCON XH 2 O has been compared with MUSICA NDACC and TCCON retrievals and has been used for MUSICA IASI and TROPOMI validation.

【 授权许可】

CC BY