Resolving the dynamics of valence-shell electrons and nuclei through laser-induced diffraction and holography

29th International Conference on Photonic, Electronic, and Atomic Collisions

Walt, Samuel G.^1 ; Ram, N Bhargava^1 ; Von Conta, Aaron^1 ; Baykusheva, Denitsa^1 ; Atala, Marcos^1 ; Wörner, Hans Jakob^1

Laboratorium für Physikalische Chemie, ETH Zürich, Zürich

8093, Switzerland^1

关键词: Electronic dynamics;    Holographic structures;    Laser induced;    Nuclear motions;    Nuclear wave packet;    Photoelectron holographies;    Time-resolved;    Valence shells;   

Others  :  https://iopscience.iop.org/article/10.1088/1742-6596/635/11/112135/pdf
DOI  :  10.1088/1742-6596/635/11/112135

来源: IOP

【 摘 要 】

We have studied a coupled electronic-nuclear wave packet in nitric oxide using time-resolved strong-field photoelectron holography and rescattering. We show that the electronic dynamics mainly appears in the holographic structures whereas nuclear motion strongly modulates the angular distribution of the rescattered photoelectrons.